On Premises Exchange Vs. Office 365 A2

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Can I use group policy to configure Outlook to connect it to 365?

 

Set up an internal DNS record for autodiscover.domain.sch.uk (whatever domain you use for emails) to point at autodiscover.outlook.com. Outlook then picks up all the settings it needs automatically when it goes through its First Run Wizard.

 

There are ways of forcing the first run wizard with registry keys if, for example, you've previously pushed a .PRF profile out through your Outlook shortcut, as I had.